hands down as of today 2015-June... its got to be NXT. I tried many other altcoin wallets and seriously. nothing compares to what the nxt devs got so far...
Below are some screenshots of the "local" native client. Many people that haven't installed the application thinks the following screenshots is a centralized website, but its not.
It's the actual live app on your computer, not a website. I was shocked when i first made this realization too.
Ethereum is also a "supposedly" promising one too. Thats assuming they release something already. You must give them credit for the hype and marketing they're capable of... But until a production release happens, its vaporware to me.